منابع مشابه
Population inversion by chirped pulses
In this paper, we analyze the condition for complete population inversion by a chirped pulse over a finite duration. The nonadiabatic transition probability is mapped in the two-dimensional parameter space of coupling strength and detuning amplitude. Asymptotic forms of the probability are derived by the interference of nonadiabatic transitions for sinusoidal and triangular pulses. The qualitat...
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The spectroscopy of large organic molecules and biomolecules in solution has been investigated using various time-resolved and frequency-resolved techniques. Of particular interest is the early response of the molecule and the solvent, which is difficult to study due to the ambiguity in assigning and differentiating inter- and intramolecular contributions to the electronic and vibrational popul...
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Direct laser acceleration of ions by short frequency chirped laser pulses is investigated theoretically. We demonstrate that intense beams of ions with a kinetic energy broadening of about 1% can be generated. The chirping of the laser pulse allows the particles to gain kinetic energies of hundreds of MeVs, which is required for hadron cancer therapy, from pulses of energies in the order of 100...
متن کاملSolvent Environment Revealed 2 by Positively Chirped Pulses
6 techniques. Of particular interest is the early response of the molecule and the 7 solvent, which is difficult to study due to the ambiguity in assigning and differ8 entiating interand intra-molecular contributions to the electronic and vibrational 9 populations and coherence. Our measurements compare the yield of fluorescence 10 for two laser dyes IR144 and IR125 as a function of chirp. Whil...
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The early optical dynamic response, resulting population, and electronic coherence are investigated experimentally and modeled theoretically for IR144 in solution. The fluorescence and stimulated emission response are studied systematically as a function of chirp. The magnitude of the chirp effect on fluorescence and stimulated emission is found to depend quadratically on pulse energy, even whe...
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ژورنال
عنوان ژورنال: Physical Review A
سال: 2011
ISSN: 1050-2947,1094-1622
DOI: 10.1103/physreva.84.033411